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Pauli was born in Vienna to a chemist Wolfgang Joseph Pauli (né Wolf Pascheles, 1869–1955) and his wife Bertha Camilla Schütz; his sister was Hertha Pauli, the writer and actress. Pauli's middle name was given in honor of his godfather, physicist Ernst Mach. Pauli's paternal grandparents were from prominent Jewish families of Prague; his great-grandfather was the Jewish publisher Wolf Pascheles. Pauli's father converted from Judaism to Roman Catholicism shortly before his marriage in 1899. Pauli's mother, Bertha Schütz, was raised in her own mother's Roman Catholic religion; her father was Jewish writer Friedrich Schütz. Pauli was raised as a Roman Catholic, although eventually he and his parents left the Church. He is considered to have been a deist and a mystic.

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